Toyota Repair Problems? Ask a Mechanic for Answers ASAP
About the only way you're going to get this to go closed is to remove the drive motor. If you remove the inner trim ring from the headliner and pull down on the headliner it will expose the drive motor that bolts to the sunroof tracks. There are 2 - 10 mm bolts that if you loosen up and pull the motor down it will disengage from the drive gear and allow you to slide the sunroof closed manually by hand. If the tracks are damaged or the cables are frozen in the tracks you will not be able to get disclosed but at least by disengaging the drive motor from the cable you have a chance of getting it closed.