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I found only one couple who died on the same day in Toledo, Ohio in 1964+/- 5 years. They were Robert L. and Shirley A. Black, both about 28 or 29, who died 14 August 1965. They were divorced at the times of their deaths. I found no copy of an obituary for Robert, but you can request one for Shirley Black of 305 1/2 Craig Street by using the following form: http://www.toledolibrary.org/obits/view1.asp?id1=360341
Both deaths were certified by the coroner and autopsies were performed. There is no news article online that mentions them.